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I was sure it was running, but I wanted a more complete answer, so I used google. This is what I found. http://www.cnn.com/2011/HEALTH/expert.q.a/09/23/ru...
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I think it mainly depends on exertion level. Nonscientifically speaking, I will say running burns more than walking. It's just harder to run.
The answer is much more complex than that. Find it here
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